"The Rose With A Broken Neck" by Danger Mouse & Daniele Luppi. Heard this whilst Lauren, Ivy and I were in the café at Spike Island this afternoon and hunted it down immediately:

On a completely different note, I've just been listening to a World Routes tribute to Cape Verdean singer Cesária Évora, featuring Tito Paris performing "Regresso" (a song he wrote for Évora). Here's the very different, but equally lovely version by Évora: